Twofold Unsymmetrical CH Functionalization of PyrDipSi-Substituted Arenes: A General Method for the Synthesis of Substituted <i>meta</i>-Halophenols

Sarkar, Dhruba; Melkonyan, Ferdinand S.; Gulevich, Anton V; Gevorgyan, Vladimir

doi:10.1002/ange.201304884

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Twofold Unsymmetrical CH Functionalization of PyrDipSi-Substituted Arenes: A General Method for the Synthesis of Substituted meta-Halophenols

Author(s): Dhruba Sarkar , Ferdinand S. Melkonyan , Anton V. Gulevich , Vladimir Gevorgyan

Publication date (Electronic): August 22 2013

Journal: Angewandte Chemie

Publisher: Wiley

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Most cited references 73

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Directed ortho metalation. Tertiary amide and O-carbamate directors in synthetic strategies for polysubstituted aromatics

Victor Snieckus (1990)

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A highly selective catalytic method for the oxidative functionalization of C-H bonds.

Allison Dick, Kami L Hull, Melanie S. Sanford (2004)

This communication describes a new and highly practical Pd(II)-catalyzed method for the regio- and chemoselective oxidative functionalization of arenes and alkanes. Carbon-hydrogen bonds of substrates that contain a variety of directing groups (e.g., pyridine, azobenzene, pyrazole, and imine derivatives) are selectively transformed into esters, ethers, and aryl-halides under mild conditions. The scope of this reaction in terms of substrate, directing group, and oxidant is described, and a preliminary catalytic cycle is proposed.

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Removable Directing Groups in Organic Synthesis and Catalysis

Géraldine Rousseau, Bernhard Breit (2011)

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Author and article information

Journal

Title: Angewandte Chemie

Abbreviated Title: Angew. Chem.

Publisher: Wiley

ISSN: 00448249

Publication date Created: October 04 2013

Publication date (Print): October 04 2013

Publication date (Electronic): August 22 2013

Volume: 125

Issue: 41

Pages: 11000-11004

Article

DOI: 10.1002/ange.201304884

SO-VID: 87b99b8f-4af3-4517-847c-7abbcc37daa4

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http://doi.wiley.com/10.1002/tdm_license_1.1

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